As far as moving from theory into actual practice, I'm just guessing, but here's my guess. A lot would depend on how severe the constriction looked. If it were my tree and I exposed a root tightly wrapped around and partially embedded in the main stem, I would cut it ever-so-carefully to minimize additional damage to the already-damaged stem. This could be tricky, because part of the root you're trying to cut will be sunk into the main stem, below the surface, so you won't be able to get at it with loppers or pruners. I would probably work at it with a small wood chisel, taking little "bites" and going very slowly as you approach the buried cambium pressed into the main stem. Once it's actually severed, I'd try to carefully pry the rest of the root out of the "groove" so the main stem will have room to fill in again over time.
Again, this is all guesswork and may well not be the problem at all, but if it is, and the encircling root is large enough, you'll have to assess how much impact it's removal will have on the tree, in term of the water it's providing. On the other hand, since you've already thinned the canopy and there's not much foliage anyway, maybe you won't have to worry about additional water loss through the foliage. Anyway, now I'm really curious to find out what the real problem is, so please keep us posted (maybe it'll turn out to be a big bunch of beetle grubs or a gopher with a taste for latex)! Pictures would be nice, too, if it's something that's clearly visible. Good luck!